大气科学
大氣科學
대기과학
CHINESE JOURNAL OF ATMOSPHERIC SCIENCES
2001年
2期
269-276
,共8页
气溶胶%硫酸盐%气粒转化
氣溶膠%硫痠鹽%氣粒轉化
기용효%류산염%기립전화
在MM5和RADM耦合的基础上,考虑了NH3的源排放,获得了NH3的时空分布、演变特征;在此基础上,讨论了气体向粒子的转化,结果表明:干气溶胶总量分布与大气中H2SO4、NH3的浓度分布有非常好的对应,富氨环境条件下,产生干气溶胶的多少是由H2SO4浓度决定的;气溶胶中的含水量与干气溶胶的浓度分布没有太多的联系,主要取决于大气中相对湿度的大小。
在MM5和RADM耦閤的基礎上,攷慮瞭NH3的源排放,穫得瞭NH3的時空分佈、縯變特徵;在此基礎上,討論瞭氣體嚮粒子的轉化,結果錶明:榦氣溶膠總量分佈與大氣中H2SO4、NH3的濃度分佈有非常好的對應,富氨環境條件下,產生榦氣溶膠的多少是由H2SO4濃度決定的;氣溶膠中的含水量與榦氣溶膠的濃度分佈沒有太多的聯繫,主要取決于大氣中相對濕度的大小。
재MM5화RADM우합적기출상,고필료NH3적원배방,획득료NH3적시공분포、연변특정;재차기출상,토론료기체향입자적전화,결과표명:간기용효총량분포여대기중H2SO4、NH3적농도분포유비상호적대응,부안배경조건하,산생간기용효적다소시유H2SO4농도결정적;기용효중적함수량여간기용효적농도분포몰유태다적련계,주요취결우대기중상대습도적대소。
By evaluating MM5 (the Fifth Generation Penn State/NCAR Mesoscale Model), RADM (Regional Acid Deposition Model) and MARS (The Model for an Aerosol Reacting System), a coupled regional photochemical model is developed to study the transformation processes from gas to particle. With this coupled model, the characteristics of spatial and temporal distribution and variation of regional tropospheric photochemical precursors, products in the northern China are studied, such as SO2, NO2, O3, H2SO4, and HNO3. On the basis of this, the ammonia emission is considered and its spatial and temporal distribution and variation are obtained. The main conclusions are: the distribution of total dry particles is strongly correlated with the emission of SO2, NO2, and NH3; the total dry aerosol amount is mainly determined by H2SO4 concentration in ammonia-rich environment; the water amount in aerosol does not have good relationship with the distribution of dry aerosol, and it is mainly determined by the relative humidity.