原子能科学技术
原子能科學技術
원자능과학기술
ATOMIC ENERGY SCIENCE AND TECHNOLOGY
2014年
7期
1159-1164
,共6页
周浩%赵永刚%李建华%金惠民
週浩%趙永剛%李建華%金惠民
주호%조영강%리건화%금혜민
铀富集度测量%峰形模型%重峰分解
鈾富集度測量%峰形模型%重峰分解
유부집도측량%봉형모형%중봉분해
uranium enrichment determination%peak shape model%deconvolution of overlapping peaks
利用铀材料γ能谱88~100 keV能区中γ、X射线重峰分解确定同位素丰度的方法,是铀同位素分析商用软件MGAU、MGA++等的核心技术。本文建立了γ、X射线峰形模型,提出了效率拟合因子修正效率的方法,并自行编写了铀富集度分析程序。用 H PGe γ谱仪对两种化学形态、铀富集度范围为1.80%~90.1%的铀样品进行了测量,以验证自编程序的可行性。利用本文所编写的程序分析实验能谱,得到的芯块样品分析结果与标称值的相对偏差小于2%,粉末样品分析结果与标称值的相对偏差小于1%。
利用鈾材料γ能譜88~100 keV能區中γ、X射線重峰分解確定同位素豐度的方法,是鈾同位素分析商用軟件MGAU、MGA++等的覈心技術。本文建立瞭γ、X射線峰形模型,提齣瞭效率擬閤因子脩正效率的方法,併自行編寫瞭鈾富集度分析程序。用 H PGe γ譜儀對兩種化學形態、鈾富集度範圍為1.80%~90.1%的鈾樣品進行瞭測量,以驗證自編程序的可行性。利用本文所編寫的程序分析實驗能譜,得到的芯塊樣品分析結果與標稱值的相對偏差小于2%,粉末樣品分析結果與標稱值的相對偏差小于1%。
이용유재료γ능보88~100 keV능구중γ、X사선중봉분해학정동위소봉도적방법,시유동위소분석상용연건MGAU、MGA++등적핵심기술。본문건립료γ、X사선봉형모형,제출료효솔의합인자수정효솔적방법,병자행편사료유부집도분석정서。용 H PGe γ보의대량충화학형태、유부집도범위위1.80%~90.1%적유양품진행료측량,이험증자편정서적가행성。이용본문소편사적정서분석실험능보,득도적심괴양품분석결과여표칭치적상대편차소우2%,분말양품분석결과여표칭치적상대편차소우1%。
T he method w hich is used to determine uranium enrichment by deconvoluting complex peak clusters in 88-100 keV region of γ/X spectrum of uranium materials is the key technique of some uranium enrichment determination software ,such as MGAU , MGA + + ,etc .According to the basic principle of this method ,a code to analyze the spectrum was written ,in which peak shape model of γ/X ray was built to fit the spec-trum and efficiency fitting factor was developed to make efficiency correction . Two types of uranium samples with enrichment ranging from 1.80% to 90.1% were meas-ured by a HPGe detector and analyzed by the code . For the samples measured , the uranium enrichment was determined with relative deviation of about 2% for pellet and 1% for pow der samples .